The 'Guilt' dubstep-crossover band will play backed by live musicians for the first time at the festival which will also see performances from Tinie Tempah, Alex Metric, Swedish House Mafia DJ Steve Angello, Eric Prydz, Underworld and Pendulum.
Nero said: "GlobalGathering is the mother of all dance festivals, and we can't wait to perform our full live show to what we know will be a really explosive crowd."
Tinie will be taking to the stage for the second time in as many years, following his breakthrough show at last year's festival - which was at the time one of the biggest crowds he had ever played to.
Alongside the larger performers are a number of smaller stages showcasing some of the UK's more underground talent including the Godskitchen, Metropolis and RISE Arenas.
GlobalGathering 2011 takes place on July 29 and 30 at Long Marston Airfield, Stratford-Upon-Avon in England. For more information or tickets please visit www.globalgathering.com