The 25 year old was detained by police officers for a yet-to-be revealed crime.
In a video posted to his Vine.com account, he says, "This is what you get for shooting in Times Square. Getting booked at a police station, that's what you get."
Overstreet has not released any further details about the arrest, but he has tweeted, "My statement is coming shortly!"
He was filming a scene with co-star Darren Criss when cops swooped.